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Global distribution of sea salt aerosols: new constraints from in situ and remote sensing observations
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Jaeglé L.; Quinn P.K.; Bates T.S.; et al. - Copernicus GmbH, 2011We combine in situ measurements of sea salt aerosols (SS) from open ocean cruises and ground-based stations together with aerosol optical depth (AOD) observations from MODIS and AERONET, and the GEOS-Chem global chemical transport model to provide new constraints on SS emissions over the world's oceans. We find that the GEOS-Chem model using the Gong (2003) source function overestimates cruise observations of coarse mode SS mass concentrations by factors of 2–3 at high wind speeds over the cold waters of the Southern, North Pacific and North Atlantic Oceans. Furthermore, the model systematical ...
[article]Global distribution of sea salt aerosols: new constraints from in situ and remote sensing observations
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Available online: http://dx.doi.org/10.5194/acp-11-3137-2011
L. Jaeglé ; P.K. Quinn ; T.S. Bates ; B. Alexander ; J.-T. Lin
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 7 [04/01/2011] . - p.3137-3157We combine in situ measurements of sea salt aerosols (SS) from open ocean cruises and ground-based stations together with aerosol optical depth (AOD) observations from MODIS and AERONET, and the GEOS-Chem global chemical transport model to provide new constraints on SS emissions over the world's oceans. We find that the GEOS-Chem model using the Gong (2003) source function overestimates cruise observations of coarse mode SS mass concentrations by factors of 2–3 at high wind speeds over the cold waters of the Southern, North Pacific and North Atlantic Oceans. Furthermore, the model systematically underestimates SS over the warm tropical waters of the Central Pacific, Atlantic, and Indian Oceans. This pattern is confirmed by SS measurements from a global network of 15 island and coastal stations. The model discrepancy at high wind speeds (>6 m s −1) has a clear dependence on sea surface temperature (SST). We use the cruise observations to derive an empirical SS source function depending on both wind speed and SST. Implementing this new source function in GEOS-Chem results in improved agreement with in situ observations, with a decrease in the model bias from +64% to +33% for the cruises and from +32% to −5% for the ground-based sites. We also show that the wind speed-SST source function significantly improves agreement with MODIS and AERONET AOD, and provides an explanation for the high AOD observed over the tropical oceans. With the wind speed-SST formulation, global SS emissions show a small decrease from 5200 Mg yr−1 to 4600 Mg yr−1, while the SS burden decreases from 9.1 to 8.5 mg m−2. The spatial distribution of SS, however, is greatly affected, with the SS burden increasing by 50% in the tropics and decreasing by 40% at mid- and high-latitudes. Our results imply a stronger than expected halogen source from SS in the tropical marine boundary layer. They also imply stronger radiative forcing of SS in the tropics and a larger response of SS emissions to climate change than previously thought.
Language(s): English
Format: Digital (Free)Tags: Aerosols ; Methodology ; Observations
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Impact of model grid spacing on regional- and urban- scale air quality predictions of organic aerosol
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Stroud C.A.; Makar P.A.; Moran M.D.; et al. - Copernicus GmbH, 2011Regional-scale chemical transport model predictions of urban organic aerosol to date tend to be biased low relative to observations, a limitation with important implications for applying such models to human exposure health studies. We used a nested version of Environment Canada's AURAMS model (42- to- 15- to- 2.5-km nested grid spacing) to predict organic aerosol concentrations for a temporal and spatial domain corresponding to the Border Air Quality and Meteorology Study (BAQS-Met), an air-quality field study that took place in the southern Great Lakes region in the summer of 2007. The use o ...
[article]Impact of model grid spacing on regional- and urban- scale air quality predictions of organic aerosol
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Available online: http://dx.doi.org/10.5194/acp-11-3107-2011
C.A. Stroud ; P.A. Makar ; M.D. Moran ; W. Gong ; S. Gong ; J. Zhang ; K. Hayden ; C. Mihele ; J.R. Brook ; J.P.D. Abbatt ; J.G. Slowik
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 7 [04/01/2011] . - p.3107-3118Regional-scale chemical transport model predictions of urban organic aerosol to date tend to be biased low relative to observations, a limitation with important implications for applying such models to human exposure health studies. We used a nested version of Environment Canada's AURAMS model (42- to- 15- to- 2.5-km nested grid spacing) to predict organic aerosol concentrations for a temporal and spatial domain corresponding to the Border Air Quality and Meteorology Study (BAQS-Met), an air-quality field study that took place in the southern Great Lakes region in the summer of 2007. The use of three different horizontal grid spacings allowed the influence of this parameter to be examined. A domain-wide average for the 2.5-km domain and a matching 15-km subdomain yielded very similar organic aerosol averages (4.8 vs. 4.3 μg m−3, respectively). On regional scales, secondary organic aerosol dominated the organic aerosol composition and was adequately resolved by the 15-km model simulation. However, the shape of the organic aerosol concentration histogram for the Windsor urban station improved for the 2.5-km simulation relative to those from the 42- and 15-km simulations. The model histograms for the Bear Creek and Harrow rural stations were also improved in the high concentration "tail" region. As well the highest-resolution model results captured the midday 4 July organic-aerosol plume at Bear Creek with very good temporal correlation. These results suggest that accurate simulation of urban and large industrial plumes in the Great Lakes region requires the use of a high-resolution model in order to represent urban primary organic aerosol emissions, urban VOC emissions, and the secondary organic aerosol production rates properly. The positive feedback between the secondary organic aerosol production rate and existing organic mass concentration is also represented more accurately with the highest-resolution model. Not being able to capture these finer-scale features may partly explain the consistent negative bias reported in the literature when urban-scale organic aerosol evaluations are made using coarser-scale chemical transport models.
Language(s): English
Format: Digital (Free)Tags: Aerosols ; Methodology ; Urban zone ; Weather forecasting ; Air quality ; Research
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A new method for retrieval of the extinction coefficient of water clouds by using the tail of the CALIOP signal
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Li J.; Hu Y.; Huang J.; et al. - Copernicus GmbH, 2011A method is developed based on Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) level 1 attenuated backscatter profile data for deriving the mean extinction coefficient of water droplets close to cloud top. The method is applicable to low level (cloud top <2 km), opaque water clouds in which the lidar signal is completely attenuated beyond about 100 m of penetration into the cloud. The photo multiplier tubes (PMTs) of the 532 nm detectors (parallel and perpendicular polarizations) of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) both exhibit a non-id ...
[article]A new method for retrieval of the extinction coefficient of water clouds by using the tail of the CALIOP signal
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Available online: http://dx.doi.org/10.5194/acp-11-2903-2011
J. Li ; Y. Hu ; J. Huang ; K. Stamnes ; Y. Yi ; S. Stamnes
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2903-2916A method is developed based on Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) level 1 attenuated backscatter profile data for deriving the mean extinction coefficient of water droplets close to cloud top. The method is applicable to low level (cloud top <2 km), opaque water clouds in which the lidar signal is completely attenuated beyond about 100 m of penetration into the cloud. The photo multiplier tubes (PMTs) of the 532 nm detectors (parallel and perpendicular polarizations) of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) both exhibit a non-ideal recovery of the lidar signal after striking a strongly backscattering target (such as water cloud or surface). Therefore, the effects of any transient responses of CALIOP on the attenuated backscatter profile of the water cloud must first be removed in order to obtain a reliable (validated) attenuated backscatter profile. Then, the slope of the exponential decay of the validated water cloud attenuated backscatter profile, and the multiple scattering factor are used for deriving the mean extinction coefficient of low-level water cloud droplets close to cloud top. This novel method was evaluated and compared with the previous method which combined the cloud effective radius (3.7-μm) reported by MODIS with the lidar depolarization ratios measured by CALIPSO to estimate the mean extinction coefficient. Statistical results show that the extinction coefficients derived by the new method based on CALIOP alone agree reasonbably well with those obtained in the previous study using combined CALIOP and MODIS data. The mean absolute relative difference in extinction coefficient is about 13.4%. An important advantage of the new method is that it can be used to derive the extinction coefficient also during night time, and it is also applicable when multi-layered clouds are present. Overall, the stratocumulus dominated regions experience larger day-night differences which are all negative and seasonal. However, a contrary tendency consisted in the global mean values. The global mean cloud water extinction coefficients during different seasons range from 26 to 30 km−1, and the differences between day and night time are all positive and small (about 1–2 km−1). In addition, the global mean layer-integrated depolarization ratios of liquid water clouds during different seasons range from 0.2 to 0.23, and the differences between day and night also are small, about 0.01.
Language(s): English
Format: Digital (Free)Tags: Water ; Methodology ; Water cloud ; Research
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GAW Report, 200. WMO/GAW Standard Operating Procedures for In-situ Measurements of Aerosol Mass Concentration, Light Scattering and Light Absorption
WMO/GAW Standard Operating Procedures for In-situ Measurements of Aerosol Mass Concentration, Light Scattering and Light Absorption
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Published by: WMO ; 2011
Collection(s) and Series: GAW Report- No. 200
Language(s): English
Format: Digital (Free), Hard copyTags: Observations ; Aerosols ; Measure ; Methodology ; Global Atmosphere Watch Programme (GAW) ; GAW 200
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Assessing the role of economic instruments in a policy mix for biodiversity conservation and ecosystem services provision : a review of some methodological challenges
In the context of the EU 2010 goal of halting biodiversity loss, researchers have been called upon to evaluate the role of economic instruments for cost-effective decision-making, as well as non-market methods to assess their benefits. This paper reviews a number of methodological challenges of evaluating and designing economic instruments aimed at biodiversity conservation and ecosystem services provision in an existing policy mix. The study draws on experiences from Brazil and Costa Rica.
Assessing the role of economic instruments in a policy mix for biodiversity conservation and ecosystem services provision: a review of some methodological challenges
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Available online: http://bioecon-network.org/pages/11th_2009/Barton.pdf
D.N. Barton ; I. Ring ; G. Rusch ; Norwegian Institute for Nature Research
Published by: NINA ; 2010In the context of the EU 2010 goal of halting biodiversity loss, researchers have been called upon to evaluate the role of economic instruments for cost-effective decision-making, as well as non-market methods to assess their benefits. This paper reviews a number of methodological challenges of evaluating and designing economic instruments aimed at biodiversity conservation and ecosystem services provision in an existing policy mix. The study draws on experiences from Brazil and Costa Rica.
Language(s): English
Format: Digital (Free) (ill.)Tags: Environment and landscape ; Economics ; Biodiversity ; Methodology ; Costa Rica ; Brazil
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WMO Global Operational Network in Support of Multi-Hazard Early Warning Systems [Poster] : natural hazards do not need to lead to disasters
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GAW Report, 148. Report of the eleventh WMO/IAEA Meeting of Experts on Carbon Dioxide Concentration and Related Tracer Measurement Techniques
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39 - February 2000 - Study on the objective forecasting techniques
is an issue of 気象研究所技術報告. Meteorological Research Institute, 2000
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GAW Report, 121. Report of the eighth WMO Meeting of Experts on Carbon Dioxide Concentration and Isotopic Measurement Techniques
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If the Price is Right- Development of a Methodology for Valuing Hydrologic Data : In 23rd Hydrology and Water Resources Symposium
Increasing restrictions on public funding for hydrologic data collection, and a trend over recent years for data collection activities to be driven by current specific use projects, have highlighted more than ever before the need to systematically assess the value of the benefits derived from the collection of hydrologic data. A most important aspect of this need is to make sensible, realistic estimates of the economic value of sll,ch benefits in dollar terms for current as well as for future uses of hydrologic data. Previous attempts to achieve this have been of limited practical application, ...
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Technical reports in hydrology and water resources, 51. Management overview of flood forecasting systems (MOFFS), Version 3
A points weighting method which enables the facilities and performance of individual flood forecasting systems to be simply described, monitored and assessed for management purposes.
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Informes técnicos de hydrología y recursos hídricos, 51. Análisis de la gestión de los sistemas de predicción de crecidas (MOFFS), versión 3
Método de puntuación que permite describir, controlar y evaluar con fines de gestión las instalaciones y el rendimiento de los distintos sistemas de predicción de crecidas.
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Rapports techniques sur l'hydrologie et les ressources en eau, 51. Evaluation globale de la gestion des systèmes de prévision des crues (MOFFS), Version 3
Méthode simple d'évaluation par points permettant de décrire, de contrôler et d'évaluer les outils d'un système individuel de prévision de crue et leur efficacité en vue de sa gestion.
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