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Available online: http://klima.hr/klima_e.php?id=atlas_vjetra_e
Published by: Meteorological and Hydrological Service ; 2012
Language(s): English
Format: Digital (Free) (ill., maps)Tags: Observations ; Wind ; Atlas ; Croatia
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Финансовые рынки стимулируют потребность в моделях климата
Оперативное прогнозирование климата завоевывает позиции в качестве самой современной, активно развивающейся области климатического обслуживания для финансового сектора.
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in Бюллетень > TOM 60(1) (2011 г.) . - p.34-37Оперативное прогнозирование климата завоевывает позиции в качестве самой современной, активно развивающейся области климатического обслуживания для финансового сектора.
Language(s): Russian; Other Languages: English, French, Spanish
Format: Digital (Free), Hard copyTags: Climate ; Climate model ; Information management ; Modelling
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Integración de los analistas financieros y científicos
Los planificadores nacionales están buscando inversores privados que contribuyan a financiar los planes de desarrollo basados en unas bajas emisiones de carbono.
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in Boletín > Vol.60(1) (2011) . - p.34-37Los planificadores nacionales están buscando inversores privados que contribuyan a financiar los planes de desarrollo basados en unas bajas emisiones de carbono.
Language(s): Spanish; Other Languages: English, French, Russian
Format: Digital (Free), Hard copyTags: Climate ; Climate model ; Information management ; Modelling ; Economics
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Algunas preguntas frecuentes: El Marco Mundial para los Servicios Climáticos
Boletín, Vol.60(1). OMM, 2011¿Qué tienen en común un ingeniero experto en aire acondicionado, un agricultor y un planificador urbanístico?
Todos ellos utilizan la información climática para hacer bien su trabajo.
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in Boletín > Vol.60(1) (2011) . - p.5-8¿Qué tienen en común un ingeniero experto en aire acondicionado, un agricultor y un planificador urbanístico?
Todos ellos utilizan la información climática para hacer bien su trabajo.Language(s): Spanish; Other Languages: English, French, Russian
Format: Digital (Free), Hard copyTags: Climate ; National Meteorological and Hydrological Service (NMHS)
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in ECMWF Newsletter > Number 128 (Summer 2011) . - p.17-22Language(s): English
Format: DigitalTags: Observations ; Satellite ; Forecast error
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Vol. 55, No. 1 - March 2011
is an issue of Antarctic Record. Scholarly and Academic Information Navigator (CiNii), 2011Contains:
-Activity report of the 40th Japanese Antarctic Research Expedition wintering party in 1999-2000
-Activities of the summer operation of the 51st Japanese Antarctic Research Expedition (JARE-51) in 2009-2010
-Observations of atmospheric dimethyl sulfide in the Southern Ocean during a cruise on the research vessel Umitakamaru in 2008-2009
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Have primary emission reduction measures reduced ozone across Europe?: An analysis of European rural background ozone trends 1996–2005
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 6. Wilson R.C.; Fleming Z.L.; Monks P.S.; et al. - Copernicus GmbH, 2011National and European legislation over the past 20 years, and the modernisation or removal of industrial sources, have significantly reduced European ozone precursor emissions. This study quantifies observed and modelled European ozone annual and seasonal linear trends from 158 harmonised rural background monitoring stations over a constant time period of a decade (1996–2005). Mean ozone concentrations are investigated, in addition to the ozone 5th percentiles as a measure of the baseline or background conditions, and the 95th percentiles that are representative of the peak concentration level ...
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Los servicios climáticos pueden invertir la espiral descendente. Caso práctico: Haití
Los servicios climáticos son fundamentales para respaldar el esfuerzo de Haití de reconstruir el país, tras las devastadoras consecuencias del terremoto que tuvo lugar a principios de este año.
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Mejora en la alerta de ciclones. Caso práctico: Filipinas
Mejorar la predicción de los ciclones es uno de los objetivos de la investigación meteorológica internacional. Este caso práctico de un tifón de 2009 que estuvo a punto de impactar sobre Filipinas ofrece una perspectiva del alcance de la predicción por conjuntos.
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Las predicciones se volverán más sutiles: Entrevista con Eugenia Kalnay
Boletín, Vol. 59(2). OMM, 2011El hecho de contar con mejores predicciones representa un importantísimo logro científico, y estas predicciones se tornarán más sutiles, tal y como defiende Eugenia Kalnay, ganadora del Premio de la Organización Meteorológica Internacional de 2009. La OMM ha estado en primera línea de la colaboración para hacer que esto sea posible. La obtención de noticias acerca de predicciones para la audiencia adecuada constituye el siguiente desafío.
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Creating a volunteer observing network: interview with Nolan Doesken and Henry Reges
Bulletin, Vol. 60 (1). WMO, 2011
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US Weather Satellites saw tornado swarm coming 5 days out
SAN FRANCISCO — Five days before approximately 200 tornadoes swept through six states in the Southeastern United States between April 25 and April 28, local meteorologists were alerted to the possibility of unusually severe weather by National Oceanic and Atmospheric Administration (NOAA) satellite data.
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Evaluation of the accuracy of analysis tools for atmospheric new particle formation
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Korhonen H.; Sihto S.-L.; Kerminen V.-M.; et al. - Copernicus GmbH, 2011Several mathematical tools have been developed in recent years to analyze new particle formation rates and to estimate nucleation rates and mechanisms at sub-3 nm sizes from atmospheric aerosol data. Here we evaluate these analysis tools using 1239 numerical nucleation events for which the nucleation mechanism and formation rates were known exactly. The accuracy of the estimates of particle formation rate at 3 nm (J3) showed significant sensitivity to the details of the analysis, i.e. form of equations used and assumptions made about the initial size of nucleating clusters, with the fraction o ...
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Analysis of number size distributions of tropical free tropospheric aerosol particles observed at Pico Espejo (4765 m a.s.l.), Venezuela
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Schmeissner T.; Krejci R.; Ström J.; et al. - Copernicus GmbH, 2011The first long-term measurements of aerosol number and size distributions in South-American tropical free troposphere (FT) were performed from March 2007 until March 2009. The measurements took place at the high altitude Atmospheric Research Station Alexander von Humboldt. The station is located on top of the Sierra Nevada mountain ridge at 4765 m a.s.l. nearby the city of Mérida, Venezuela. Aerosol size distribution and number concentration data was obtained with a custom-built Differential Mobility Particle Sizer (DMPS) system and a Condensational Particle Counter (CPC). The analysis of the ...
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Dependence of the single-scattering properties of small ice crystals on idealized shape models
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Um J.; McFarquhar G.M. - Copernicus GmbH, 2011The projections of small ice crystals (with maximum dimension <50 μm) appear quasi-circular when imaged by probes on aircraft flying through cloud. Therefore, idealized models constructed to calculate their single-scattering properties have included quasi-spherical models such as Chebyshev particles, Gaussian random spheres, and droxtals. Recently, an ice analogue grown from sodium fluorosilicate solution on a glass substrate, with several columns emanating from a common center of mass, was shown to be quasi-circular when imaged by state-of-the-art cloud probes. In this study, a new idealized ...
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Microphysical and radiative effects of aerosols on warm clouds during the Amazon biomass burning season as observed by MODIS: impacts of water vapor and land cover
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Ten Hoeve J.E.; Remer L.A.; Jacobson M.Z. - Copernicus GmbH, 2011Aerosol, cloud, water vapor, and temperature profile data from the Moderate Resolution Imaging Spectroradiometer (MODIS) are utilized to examine the impact of aerosols on clouds during the Amazonian biomass burning season in Rondônia, Brazil. It is found that increasing background column water vapor (CWV) throughout this transition season between the Amazon dry and wet seasons likely exerts a strong effect on cloud properties. As a result, proper analysis of aerosol-cloud relationships requires that data be stratified by CWV to account better for the influence of background meteorological vari ...
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Synergetic monitoring of Saharan dust plumes and potential impact on surface: a case study of dust transport from Canary Islands to Iberian Peninsula
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Córdoba-Jabonero C.; Sorribas M.; Guerrero-Rascado J.L.; et al. - Copernicus GmbH, 2011The synergetic use of meteorological information, remote sensing both ground-based active (lidar) and passive (sun-photometry) techniques together with backtrajectory analysis and in-situ measurements is devoted to the characterization of dust intrusions. A case study of air masses advected from the Saharan region to the Canary Islands and the Iberian Peninsula, located relatively close and far away from the dust sources, respectively, was considered for this purpose. The observations were performed over three Spanish geographically strategic stations within the dust-influenced area along a co ...
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African biomass burning plumes over the Atlantic: aircraft based measurements and implications for H2SO4 and HNO3 mediated smoke particle activation
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Fiedler V.; Arnold F.; Ludmann S.; et al. - Copernicus GmbH, 2011Airborne measurements of trace gases and aerosol particles have been made in two aged biomass burning (BB) plumes over the East Atlantic (Gulf of Guinea). The plumes originated from BB in the Southern-Hemisphere African savanna belt. On the day of our measurements (13 August 2006), the plumes had ages of about 10 days and were respectively located in the middle troposphere (MT) at 3900–5500 m altitude and in the upper troposphere (UT) at 10 800–11 200 m. Probably, the MT plume was lifted by dry convection and the UT plume was lifted by wet convection. In the more polluted MT-plume, numerous me ...
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Global distribution of sea salt aerosols: new constraints from in situ and remote sensing observations
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Jaeglé L.; Quinn P.K.; Bates T.S.; et al. - Copernicus GmbH, 2011We combine in situ measurements of sea salt aerosols (SS) from open ocean cruises and ground-based stations together with aerosol optical depth (AOD) observations from MODIS and AERONET, and the GEOS-Chem global chemical transport model to provide new constraints on SS emissions over the world's oceans. We find that the GEOS-Chem model using the Gong (2003) source function overestimates cruise observations of coarse mode SS mass concentrations by factors of 2–3 at high wind speeds over the cold waters of the Southern, North Pacific and North Atlantic Oceans. Furthermore, the model systematical ...
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Multi-scale modeling study of the source contributions to near-surface ozone and sulfur oxides levels over California during the ARCTAS-CARB period
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Huang M.; Carmichael Gregory R.; Spak S.N.; et al. - Copernicus GmbH, 2011Chronic high surface ozone (O3) levels and the increasing sulfur oxides (SOx = SO2+SO4) ambient concentrations over South Coast (SC) and other areas of California (CA) are affected by both local emissions and long-range transport. In this paper, multi-scale tracer, full-chemistry and adjoint simulations using the STEM atmospheric chemistry model are conducted to assess the contribution of local emission sourcesto SC O3 and to evaluate the impacts of transported sulfur and local emissions on the SC sulfur budgetduring the ARCTAS-CARB experiment period in 2008. Sensitivity simulations quantify c ...
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The effect of meteorological and chemical factors on the agreement between observations and predictions of fine aerosol composition in southwestern Ontario during BAQS-Met
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Markovic M.Z.; Hayden K.L.; Murphy J.G.; et al. - Copernicus GmbH, 2011The Border Air Quality and Meteorology Study (BAQS-Met) was an intensive, collaborative field campaign during the summer of 2007 that investigated the effects of transboundary pollution, local pollution, and local meteorology on air quality in southwestern Ontario. This analysis focuses on the measurements of the inorganic constituents of particulate matter with diameter of less than 1 μm (PM1), with a specific emphasis on nitrate. We evaluate the ability of AURAMS, Environment Canada's chemical transport model, to represent regional air pollution in SW Ontario by comparing modelled aerosol in ...
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Latitudinal distributions of organic nitrogen and organic carbon in marine aerosols over the western North Pacific
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Miyazaki Y.; Kawamura K.; Jung J.; et al. - Copernicus GmbH, 2011Marine aerosol samples were collected over the western North Pacific along the latitudinal transect from 44° N to 10° N in late summer 2008 for measurements of organic nitrogen (ON) and organic carbon (OC) as well as isotopic ratios of total nitrogen (TN) and total carbon (TC). Increased concentrations of methanesulfonic acid (MSA) and diethylammonium (DEA+) at 40–44° N and subtropical regions (10–20° N) together with averaged satellite chlorophyll-a data and 5-day back trajectories suggest a significant influence of marine biological activities on aerosols in these regions. ON exhibited incre ...
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The Smithsonian solar constant data revisited: no evidence for a strong effect of solar activity in ground-based insolation data
Apparent evidence for a strong signature of solar activity in ground-based insolation data was recently reported. In particular, a strong increase of the irradiance of the direct solar beam with sunspot number as well as a decline of the brightness of the solar aureole and the measured precipitable water content of the atmosphere with solar activity were presented. The latter effect was interpreted as evidence for cosmic-ray-induced aerosol formation. Here I show that these spurious results are due to a failure to correct for seasonal variations and the effects of volcanic eruptions and local ...
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Saharan and Asian dust: similarities and differences determined by CALIPSO, AERONET, and a coupled climate-aerosol microphysical model
This study compares the properties of atmospheric dust from the Saharan deserts and the Asian deserts using data from CALIPSO and AERONET during 2006 and 2007 along with simulations using a coupled climate-microphysical sectional model. Saharan deserts are largely south of 30° N, while Asian ones are primarily north of 30° N, hence they experience different meteorological regimes. Saharan dust lifting occurs all year long, primarily due to subtropical weather systems. However, Asian dust is lifted mostly in spring when mid-latitude frontal systems lead to high winds. Rainfall is more abundant ...
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Impact of model grid spacing on regional- and urban- scale air quality predictions of organic aerosol
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 7. Stroud C.A.; Makar P.A.; Moran M.D.; et al. - Copernicus GmbH, 2011Regional-scale chemical transport model predictions of urban organic aerosol to date tend to be biased low relative to observations, a limitation with important implications for applying such models to human exposure health studies. We used a nested version of Environment Canada's AURAMS model (42- to- 15- to- 2.5-km nested grid spacing) to predict organic aerosol concentrations for a temporal and spatial domain corresponding to the Border Air Quality and Meteorology Study (BAQS-Met), an air-quality field study that took place in the southern Great Lakes region in the summer of 2007. The use o ...
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The 2009–2010 Arctic polar stratospheric cloud season: a CALIPSO perspective
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 5. Pitts M.C.; Poole L.R.; Dörnbrack A.; et al. - Copernicus GmbH, 2011Spaceborne lidar measurements from CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) are used to provide a vortex-wide perspective of the 2009–2010 Arctic PSC (polar stratospheric cloud) season to complement more focused measurements from the European Union RECONCILE (reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions) field campaign. The 2009–2010 Arctic winter was unusually cold at stratospheric levels from mid-December 2009 until the end of January 2010, and was one of only ...
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Boundary layer dynamics over London, UK, as observed using Doppler lidar during REPARTEE-II
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 5. Barlow J.F.; Dunbar T.M.; Nemitz E.G.; et al. - Copernicus GmbH, 2011Urban boundary layers (UBLs) can be highly complex due to the heterogeneous roughness and heating of the surface, particularly at night. Due to a general lack of observations, it is not clear whether canonical models of boundary layer mixing are appropriate in modelling air quality in urban areas. This paper reports Doppler lidar observations of turbulence profiles in the centre of London, UK, as part of the second REPARTEE campaign in autumn 2007. Lidar-measured standard deviation of vertical velocity averaged over 30 min intervals generally compared well with in situ sonic anemometer measure ...
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Evaluation of urban surface parameterizations in the WRF model using measurements during the Texas Air Quality Study 2006 field campaign
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 5. Lee S.-H.; Kim S.-W.; Angevine W.M.; et al. - Copernicus GmbH, 2011The performance of different urban surface parameterizations in the WRF (Weather Research and Forecasting) in simulating urban boundary layer (UBL) was investigated using extensive measurements during the Texas Air Quality Study 2006 field campaign. The extensive field measurements collected on surface (meteorological, wind profiler, energy balance flux) sites, a research aircraft, and a research vessel characterized 3-dimensional atmospheric boundary layer structures over the Houston-Galveston Bay area, providing a unique opportunity for the evaluation of the physical parameterizations. The m ...
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Continuous 1064/532 nm Lidar Measurements (CORALNet-UBC) in Vancouver, British Columbia: Selected Results from a Year of Operation
Atmosphere-ocean, Vol. 49 No.1. McKendry I.G.; Strawbridge K.B.; Jones A. - Canadian Meteorological and Oceanographic Society, 2011CORALNet-UBC was installed in April 2008 as a “proof of concept” and the first facility in a proposed cross-Canada network of similar lidars. Despite its location on the wet West Coast of Canada, data recovery ranged from a low of 45% of the total time in December, when heavy snowfall interrupted operations, to a high of 90% in July. The facility has been a spectacular success in terms of its operational characteristics (as measured by data recovery), the range of phenomena observed and the research that it has spawned. Examples are provided of the types of phenomena observed since its initial ...
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Ozone production in remote oceanic and industrial areas derived from ship based measurements of peroxy radicals during TexAQS 2006
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Sommariva R.; Brown S.S.; Roberts J.M.; et al. - Copernicus GmbH, 2011During the Texas Air Quality Study II (TexAQS 2006) campaign, a PEroxy Radical Chemical Amplifier (PERCA) was deployed on the NOAA research vessel R/V Brown to measure total peroxy radicals (HO2+Σ RO2). Day-time mixing ratios of HO2+Σ RO2 between 25 and 110 ppt were observed throughout the study area – the Houston/Galveston region and the Gulf coast of the US – and analyzed in relation to measurements of nitrogen oxides, volatile organic compounds (VOC) and photolysis rates to assess radical sources and sinks in the region.
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Optical properties of pristine ice crystals in mid-latitude cirrus clouds: a case study during CIRCLE-2 experiment
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Gayet J.-F.; Mioche G.; Shcherbakov V.; et al. - Copernicus GmbH, 2011In this paper, we describe in situ observations of mid-latitude cirrus cloud band carried out on 16 May 2007 during the CIRCLE-2 experiment. The Polar Nephelometer and the Cloud Particle Imager (CPI) instruments with PMS FSSP-300 and 2D-C probes were used for the description of the optical and microphysical cloud properties. Two selected cloud regions are compared and discussed in detail. Significant differences in optical properties are evidenced in terms of 22° halo occurrences even though prevalent planar-plate ice crystals are observed in both cloud regions. Featureless scattering phase fu ...
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Transport analysis of ozone enhancement in Southern Ontario during BAQS-Met
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. He H.; Tarasick D.W.; Hocking W.K.; et al. - Copernicus GmbH, 2011Twice-daily ozonesondes were launched from Harrow, in southwestern Ontario, Canada, during the BAQS-Met (Border Air Quality and Meteorology Study) field campaign in June and July of 2007. A co-located radar windprofiler measured tropopause height continuously. These data, in combination with continuous surface ozone measurements and geo-statistical interpolation of satellite ozone observations, present a consistent picture and indicate that a number of significant ozone enhancements in the troposphere were observed that were the result of stratospheric intrusion events. The combined observatio ...
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Measurements of volatile organic compounds at a suburban ground site (T1) in Mexico City during the MILAGRO 2006 campaign: measurement comparison, emission ratios, and source attribution
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Bon D.M.; Ulbrich I.M.; de Gouw J.A.; et al. - Copernicus GmbH, 2011Volatile organic compound (VOC) mixing ratios were measured with two different instruments at the T1 ground site in Mexico City during the Megacity Initiative: Local and Global Research Observations (MILAGRO) campaign in March of 2006. A gas chromatograph with flame ionization detector (GC-FID) quantified 18 light alkanes, alkenes and acetylene while a proton-transfer-reaction ion-trap mass spectrometer (PIT-MS) quantified 12 VOC species including oxygenated VOCs (OVOCs) and aromatics. A GC separation system was used in conjunction with the PIT-MS (GC-PIT-MS) to evaluate PIT-MS measurements an ...
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Distribution and air-sea exchange of mercury (Hg) in the Yellow Sea
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Ci Z.J.; Zhang X.S.; Wang Z.W.; et al. - Copernicus GmbH, 2011The Yellow Sea, surrounded by East China and the Korea Peninsula, is a potentially important receptor for anthropogenic mercury (Hg) emissions from East Asia. However, there is little documentation about the distribution and cycle of Hg in this marine system. During the cruise covering the Yellow Sea in July 2010, gaseous elemental mercury (GEM or Hg(0)) in the atmosphere, total Hg (THg), reactive Hg (RHg) and dissolved gaseous mercury (DGM, largely Hg(0)) in the waters were measured aboard the R/V Kexue III. The mean (±SD) concentration of GEM over the entire cruise was 2.61 ± 0.50 ng m−3 (ra ...
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Evaluating a 3-D transport model of atmospheric CO2 using ground-based, aircraft, and space-borne data
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Feng L.; Palmer P.I.; Yang Y.; et al. - Copernicus GmbH, 2011We evaluate the GEOS-Chem atmospheric transport model (v8-02-01) of CO2 over 2003–2006, driven by GEOS-4 and GEOS-5 meteorology from the NASA Goddard Global Modeling and Assimilation Office, using surface, aircraft and space-borne concentration measurements of CO2. We use an established ensemble Kalman Filter to estimate a posteriori biospheric+biomass burning (BS + BB) and oceanic (OC) CO2 fluxes from 22 geographical regions, following the TransCom-3 protocol, using boundary layer CO2 data from a subset of GLOBALVIEW surface sites. Global annual net BS + BB + OC CO2 fluxes over 2004–2006 for ...
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Sensitivity of mesoscale model urban boundary layer meteorology to the scale of urban representation
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Flagg D.D.; Taylor P.A. - Copernicus GmbH, 2011Mesoscale modeling of the urban boundary layer requires careful parameterization of the surface due to its heterogeneous morphology. Model estimated meteorological quantities, including the surface energy budget and canopy layer variables, will respond accordingly to the scale of representation. This study examines the sensitivity of the surface energy balance, canopy layer and boundary layer meteorology to the scale of urban surface representation in a real urban area (Detroit-Windsor (USA-Canada)) during several dry, cloud-free summer periods. The model used is the Weather Research and Forec ...
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Chemical composition and mixing-state of ice residuals sampled within mixed phase clouds
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Ebert M.; Worringen A.; Benker N.; et al. - Copernicus GmbH, 2011During an intensive campaign at the high alpine research station Jungfraujoch, Switzerland, in February/March 2006 ice particle residuals within mixed-phase clouds were sampled using the Ice-counterflow virtual impactor (Ice-CVI). Size, morphology, chemical composition, mineralogy and mixing state of the ice residual and the interstitial (i.e., non-activated) aerosol particles were analyzed by scanning and transmission electron microscopy. Ice nuclei (IN) were identified from the significant enrichment of particle groups in the ice residual (IR) samples relative to the interstitial aerosol. In ...
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Sources of carbonaceous aerosol in the Amazon basin
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Gilardoni S.; Vignati E.; Marmer E.; et al. - Copernicus GmbH, 2011The quantification of sources of carbonaceous aerosol is important to understand their atmospheric concentrations and regulating processes and to study possible effects on climate and air quality, in addition to develop mitigation strategies.
In the framework of the European Integrated Project on Aerosol Cloud Climate Interactions (EUCAARI) fine (Dp < 2.5 μm) and coarse (2.5 μm < Dp <10 μm) aerosol particles were sampled from February to June (wet season) and from August to September (dry season) 2008 in the central Amazon basin. The mass of fine particles averaged 2.4 μg m−3 duri ...
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Characteristics of CALIOP attenuated backscatter noise: implication for cloud/aerosol detection
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Wu D.L.; Chae J.H.; Lambert A.; et al. - Copernicus GmbH, 2011A research algorithm is developed for noise evaluation and feature detection of the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Level 1 (L1) backscatter data with an emphasis on cloud/aerosol features in the upper troposphere and lower stratosphere (UT/LS). CALIOP measurement noise of the version v2.01 and v2.02 L1 backscatter data aggregated to (5 km) horizontal resolution is analyzed with two approaches in this study. One is to compare the observed and modeled molecular scatter profiles by scaling the modeled profile (with a fitted scaling factor α) to the observed clear-sky ba ...
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Long-term analysis of carbon dioxide and methane column-averaged mole fractions retrieved from SCIAMACHY
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Schneising O.; Buchwitz M.; Reuter M.; et al. - Copernicus GmbH, 2011Carbon dioxide (CO2) and methane (CH4) are the two most important anthropogenic greenhouse gases contributing to global climate change. SCIAMACHY onboard ENVISAT (launch 2002) was the first and is now with TANSO onboard GOSAT (launch 2009) one of only two satellite instruments currently in space whose measurements are sensitive to CO2 and CH4 concentration changes in the lowest atmospheric layers where the variability due to sources and sinks is largest.
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Representation of tropical deep convection in atmospheric models – Part 1: Meteorology and comparison with satellite observations
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Russo M.R.; Marécal V.; Hoyle C.R.; et al. - Copernicus GmbH, 2011Fast convective transport in the tropics can efficiently redistribute water vapour and pollutants up to the upper troposphere. In this study we compare tropical convection characteristics for the year 2005 in a range of atmospheric models, including numerical weather prediction (NWP) models, chemistry transport models (CTMs), and chemistry-climate models (CCMs). The model runs have been performed within the framework of the SCOUT-O3 (Stratospheric-Climate Links with Emphasis on the Upper Troposphere and Lower Stratosphere) project. The characteristics of tropical convection, such as seasonal c ...
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Atmospheric emissions from vegetation fires in Portugal (1990–2008): estimates, uncertainty analysis, and sensitivity analysis
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Rosa I.M.D.; Pereira J.M.C.; Tarantola S. - Copernicus GmbH, 2011Atmospheric emissions from wildfires in Portugal were estimated yearly over the period 1990–2008 using Landsat-based burnt area maps and land cover maps, national forest inventory data, biometric models, and literature review data. Emissions were calculated as the product of area burnt, biomass loading per unit area, combustion factor, and emission factor, using land cover specific values for all variables. Uncertainty associated with each input variable was quantified with a probability density function or a standard deviation value. Uncertainty and sensitivity analysis of estimates were perf ...
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Concurrent observations of atomic iodine, molecular iodine and ultrafine particles in a coastal environment
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Mahajan A.S.; Sorribas M.; Gómez Martín J.C.; et al. - Copernicus GmbH, 2011Simultaneous measurements of atomic iodine (I), molecular iodine (I2) and ultrafine particles were made at O Grove, Galicia (42.50° N, 8.87° W), on the northwest coast of Spain. The observations show a strong tidal signature, and indicate that the most probable sources of reactive iodine species are the exposed macroalgae during low tide. For the first time, I2 and I were concurrently measured revealing a high average I2/I ratio of ~32, which is higher than previously inferred by modelling studies. A 1-dimensional photochemical model is employed to simulate the observations showing that the hi ...
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The effect of H2SO4 – amine clustering on chemical ionization mass spectrometry (CIMS) measurements of gas-phase sulfuric acid
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Kurtén T.; Petäjä T.; Smith J.; et al. - Copernicus GmbH, 2011The state-of-the art method for measuring atmospheric gas-phase sulfuric acid is chemical ionization mass spectrometry (CIMS) based on nitrate reagent ions. We have assessed the possible effect of the sulfuric acid molecules clustering with base molecules on CIMS measurements using computational chemistry. From the computational data, three conclusions can be drawn. First, a significant fraction of the gas-phase sulfuric acid molecules are very likely clustered with amines if the amine concentration is around or above a few ppt. Second, some fraction of these acid-amine clusters may not be cha ...
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