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Characteristics of CALIOP attenuated backscatter noise: implication for cloud/aerosol detection
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Wu D.L.; Chae J.H.; Lambert A.; et al. - Copernicus GmbH, 2011A research algorithm is developed for noise evaluation and feature detection of the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Level 1 (L1) backscatter data with an emphasis on cloud/aerosol features in the upper troposphere and lower stratosphere (UT/LS). CALIOP measurement noise of the version v2.01 and v2.02 L1 backscatter data aggregated to (5 km) horizontal resolution is analyzed with two approaches in this study. One is to compare the observed and modeled molecular scatter profiles by scaling the modeled profile (with a fitted scaling factor α) to the observed clear-sky ba ...
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Available online: http://dx.doi.org/10.5194/acp-11-2641-2011
D.L. Wu ; J.H. Chae ; A. Lambert ; F.F. Zhang
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2641-2654A research algorithm is developed for noise evaluation and feature detection of the CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) Level 1 (L1) backscatter data with an emphasis on cloud/aerosol features in the upper troposphere and lower stratosphere (UT/LS). CALIOP measurement noise of the version v2.01 and v2.02 L1 backscatter data aggregated to (5 km) horizontal resolution is analyzed with two approaches in this study. One is to compare the observed and modeled molecular scatter profiles by scaling the modeled profile (with a fitted scaling factor α) to the observed clear-sky backscatter profiles. This scaling α value is sensitive to errors in the calibrated backscatter and the atmospheric model used. Most of the nighttime 532-nm α values are close to unity, as expected, but an abrupt drop occurred in October 2008 in the daytime 532-nm α, which is likely indicative of a problem in the v2.02 daytime calibrated data. The 1064-nm night α is generally close to 2 while its day α is ~3. The other approach to evaluate the lidar measurement noise is to use the calibrated lidar backscatter data at altitudes above 19 km. With this method, the 532-nm and 1064-nm measurement noises are analyzed and characterized individually for each profile in terms of the mean (μ) and standard deviation (σ), showing larger σ values in general over landmasses or bright surfaces during day and in radiation-hard regions during night. A significant increasing trend is evident in the nighttime 1064-nm σ, which is likely responsible for the increasing difference between the feature occurrence frequencies (532-nm vs. 1064-nm) derived from this study. For feature detection with the research algorithm, we apply a σ–based method to the aggregated L1 data. The derived morphology of feature occurrence frequency is in general agreement with that obtained from the Level 2 (L2) 05 km_CLAY+05 km_ALAY products at 5 km horizontal resolution. Finally, a normalized probability density function (PDF) method is employed to evaluate the day-night backscatter data in which noise levels are largely different. CALIOP observations reveal a higher probability of daytime cloud/aerosol occurrence than nighttime in the tropical UT/LS region for 532-nm total backscatters >0.01 km−1 sr−1.
Language(s): English
Format: Digital (Free)Tags: Aerosols ; Atmosphere ; Observations ; Research
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Cloud condensation nuclei in polluted air and biomass burning smoke near the mega-city Guangzhou, China – Part 2: Size-resolved aerosol chemical composition, diurnal cycles, and externally mixed weakly CCN-active soot particles
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Rose D.; Gunthe S.S.; Su H.; et al. - Copernicus GmbH, 2011Size-resolved chemical composition, mixing state, and cloud condensation nucleus (CCN) activity of aerosol particles in polluted mega-city air and biomass burning smoke were measured during the PRIDE-PRD2006 campaign near Guangzhou, China, using an aerosol mass spectrometer (AMS), a volatility tandem differential mobility analyzer (VTDMA), and a continuous-flow CCN counter (DMT-CCNC).
[article]Cloud condensation nuclei in polluted air and biomass burning smoke near the mega-city Guangzhou, China – Part 2: Size-resolved aerosol chemical composition, diurnal cycles, and externally mixed weakly CCN-active soot particles
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Available online: http://dx.doi.org/10.5194/acp-11-2817-2011
D. Rose ; S.S. Gunthe ; H. Su ; R.M. Garland ; H. Yang ; M. Berghof ; Y.F. Cheng ; B. Wehner ; P. Achtert ; A. Nowak ; A. Wiedensohler ; N. Takegawa ; Y. Kondo ; M. Hu ; Y. Zhang ; M.O. Andreae ; U. Pöschl
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2817-2836Size-resolved chemical composition, mixing state, and cloud condensation nucleus (CCN) activity of aerosol particles in polluted mega-city air and biomass burning smoke were measured during the PRIDE-PRD2006 campaign near Guangzhou, China, using an aerosol mass spectrometer (AMS), a volatility tandem differential mobility analyzer (VTDMA), and a continuous-flow CCN counter (DMT-CCNC).
Language(s): English
Format: Digital (Free)Tags: Aerosols ; Biomass ; Cloud condensation nuclei (CCN) ; Air pollution ; Research
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Long-term analysis of carbon dioxide and methane column-averaged mole fractions retrieved from SCIAMACHY
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Schneising O.; Buchwitz M.; Reuter M.; et al. - Copernicus GmbH, 2011Carbon dioxide (CO2) and methane (CH4) are the two most important anthropogenic greenhouse gases contributing to global climate change. SCIAMACHY onboard ENVISAT (launch 2002) was the first and is now with TANSO onboard GOSAT (launch 2009) one of only two satellite instruments currently in space whose measurements are sensitive to CO2 and CH4 concentration changes in the lowest atmospheric layers where the variability due to sources and sinks is largest.
[article]Long-term analysis of carbon dioxide and methane column-averaged mole fractions retrieved from SCIAMACHY
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Available online: http://dx.doi.org/10.5194/acp-11-2863-2011
O. Schneising ; M. Buchwitz ; M. Reuter ; J. Heymann ; H. Bovensmann ; J.P. Burrows
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2863-2880Carbon dioxide (CO2) and methane (CH4) are the two most important anthropogenic greenhouse gases contributing to global climate change. SCIAMACHY onboard ENVISAT (launch 2002) was the first and is now with TANSO onboard GOSAT (launch 2009) one of only two satellite instruments currently in space whose measurements are sensitive to CO2 and CH4 concentration changes in the lowest atmospheric layers where the variability due to sources and sinks is largest.
Language(s): English
Format: Digital (Free)Tags: Carbon dioxide (CO2) ; Methane (CH4) ; Long-range weather forecasting, long-term weather forecasting, long-range meteorological forecasting ; Research
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Photochemical processing of organic aerosol at nearby continental sites: contrast between urban plumes and regional aerosol
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Slowik J.G.; Brook J.; Chang R.Y.-W.; et al. - Copernicus GmbH, 2011As part of the BAQS-Met 2007 field campaign, Aerodyne time-of-flight aerosol mass spectrometers (ToF-AMS) were deployed at two sites in southwestern Ontario from 17 June to 11 July 2007. One instrument was located at Harrow, ON, a rural, agriculture-dominated area approximately 40 km southeast of the Detroit/Windsor/Windsor urban area and 5 km north of Lake Erie. The second instrument was located at Bear Creek, ON, a rural site approximately 70 km northeast of the Harrow site and 50 km east of Detroit/Windsor. Positive matrix factorization analysis of the combined organic mass spectral dataset ...
[article]Photochemical processing of organic aerosol at nearby continental sites: contrast between urban plumes and regional aerosol
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Available online: http://dx.doi.org/10.5194/acp-11-2991-2011
J.G. Slowik ; J. Brook ; R.Y.-W. Chang ; G.J. Evans ; K. Hayden ; C.-H. Jeong ; S.-M. Li ; J. Liggio ; P.S.K. Liu ; M. McGuire ; C. Mihele ; S. Sjostedt ; A. Vlasenko ; J.P.D. Abbatt
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2991-3006As part of the BAQS-Met 2007 field campaign, Aerodyne time-of-flight aerosol mass spectrometers (ToF-AMS) were deployed at two sites in southwestern Ontario from 17 June to 11 July 2007. One instrument was located at Harrow, ON, a rural, agriculture-dominated area approximately 40 km southeast of the Detroit/Windsor/Windsor urban area and 5 km north of Lake Erie. The second instrument was located at Bear Creek, ON, a rural site approximately 70 km northeast of the Harrow site and 50 km east of Detroit/Windsor. Positive matrix factorization analysis of the combined organic mass spectral dataset yields factors related to secondary organic aerosol (SOA), direct emissions, and a factor tentatively attributed to the reactive uptake of isoprene and/or condensation of its early generation reaction products. This is the first application of PMF to simultaneous AMS measurements at different sites, an approach which allows for self-consistent, direct comparison of the datasets. Case studies are utilized to investigate processing of SOA from (1) fresh emissions from Detroit/Windsor and (2) regional aerosol during periods of inter-site flow. A strong correlation is observed between SOA/excess CO and photochemical age as represented by the NOx/NOy ratio for Detroit/Windsor outflow. Although this correlation is not evident for more aged air, measurements at the two sites during inter-site transport nevertheless show evidence of continued atmospheric processing by SOA production. However, the rate of SOA production decreases with airmass age from an initial value of ~10.1 μg m−3 ppmvCO−1 h−1 for the first ~10 h of plume processing to near-zero in an aged airmass (i.e. after several days). The initial SOA production rate is comparable to the observed rate in Mexico City over similar timescales.
Language(s): English
Format: DigitalTags: Aerosols ; Ecology ; Environment and landscape ; Research ; Canada
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Representation of tropical deep convection in atmospheric models – Part 1: Meteorology and comparison with satellite observations
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Russo M.R.; Marécal V.; Hoyle C.R.; et al. - Copernicus GmbH, 2011Fast convective transport in the tropics can efficiently redistribute water vapour and pollutants up to the upper troposphere. In this study we compare tropical convection characteristics for the year 2005 in a range of atmospheric models, including numerical weather prediction (NWP) models, chemistry transport models (CTMs), and chemistry-climate models (CCMs). The model runs have been performed within the framework of the SCOUT-O3 (Stratospheric-Climate Links with Emphasis on the Upper Troposphere and Lower Stratosphere) project. The characteristics of tropical convection, such as seasonal c ...
[article]Representation of tropical deep convection in atmospheric models – Part 1: Meteorology and comparison with satellite observations
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Available online: http://dx.doi.org/10.5194/acp-11-2765-2011
M.R. Russo ; V. Marécal ; C.R. Hoyle ; J. Arteta ; C. Chemel ; M.P. Chipperfield ; O. Dessens ; W. Feng ; J.S. Hosking ; P.J. Telford ; O. Wild ; X. Yang ; J.A. Pyle
in Atmospheric Chemistry and Physics (ACP) > Vol. 11. N° 3 [03/01/2011] . - p.2765-2786Fast convective transport in the tropics can efficiently redistribute water vapour and pollutants up to the upper troposphere. In this study we compare tropical convection characteristics for the year 2005 in a range of atmospheric models, including numerical weather prediction (NWP) models, chemistry transport models (CTMs), and chemistry-climate models (CCMs). The model runs have been performed within the framework of the SCOUT-O3 (Stratospheric-Climate Links with Emphasis on the Upper Troposphere and Lower Stratosphere) project. The characteristics of tropical convection, such as seasonal cycle, land/sea contrast and vertical extent, are analysed using satellite observations as a benchmark for model simulations. The observational datasets used in this work comprise precipitation rates, outgoing longwave radiation, cloud-top pressure, and water vapour from a number of independent sources, including ERA-Interim analyses. Most models are generally able to reproduce the seasonal cycle and strength of precipitation for continental regions but show larger discrepancies with observations for the Maritime Continent region. The frequency distribution of high clouds from models and observations is calculated using highly temporally-resolved (up to 3-hourly) cloud top data. The percentage of clouds above 15 km varies significantly between the models. Vertical profiles of water vapour in the upper troposphere-lower stratosphere (UTLS) show large differences between the models which can only be partly attributed to temperature differences. If a convective plume reaches above the level of zero net radiative heating, which is estimated to be ~15 km in the tropics, the air detrained from it can be transported upwards by radiative heating into the lower stratosphere. In this context, we discuss the role of tropical convection as a precursor for the transport of short-lived species into the lower stratosphere.
Language(s): English
Format: Digital (Free)Tags: Atmospheric circulation ; Chemical model of climate ; Modelling ; Observations ; Numerical weather prediction ; Research ; Satellite
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The effect of H2SO4 – amine clustering on chemical ionization mass spectrometry (CIMS) measurements of gas-phase sulfuric acid
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Kurtén T.; Petäjä T.; Smith J.; et al. - Copernicus GmbH, 2011The state-of-the art method for measuring atmospheric gas-phase sulfuric acid is chemical ionization mass spectrometry (CIMS) based on nitrate reagent ions. We have assessed the possible effect of the sulfuric acid molecules clustering with base molecules on CIMS measurements using computational chemistry. From the computational data, three conclusions can be drawn. First, a significant fraction of the gas-phase sulfuric acid molecules are very likely clustered with amines if the amine concentration is around or above a few ppt. Second, some fraction of these acid-amine clusters may not be cha ...
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A new method for retrieval of the extinction coefficient of water clouds by using the tail of the CALIOP signal
Atmospheric Chemistry and Physics (ACP), Vol. 11. N° 3. Li J.; Hu Y.; Huang J.; et al. - Copernicus GmbH, 2011A method is developed based on Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) level 1 attenuated backscatter profile data for deriving the mean extinction coefficient of water droplets close to cloud top. The method is applicable to low level (cloud top <2 km), opaque water clouds in which the lidar signal is completely attenuated beyond about 100 m of penetration into the cloud. The photo multiplier tubes (PMTs) of the 532 nm detectors (parallel and perpendicular polarizations) of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) both exhibit a non-id ...
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Volume 89, No.1 - February 2011
is an issue of Journal of the Meteorological Society of Japan. Meteorological Society of Japan, 2011
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Anno 68 N°3 - Luglio-settembre 2008
is an issue of Rivista di Meteorologia. Organo del Servizio Meteorologico dell'Aeronautica, 2011Contiene tali:
- Il caldo anomalo del 2003 in Italia: anomalie climatiche ed
inquinamento da ozono
- HSAF - Hydrology Satellite Application Facilities: un progetto
europeo con finalità di servizio e impiego operativo
- Nuovo approccio alle previsioni stagionali: analisi
- Simulazione del Meteosat Third Generation Lightning Imager
attraverso dati reali rilevati dal satellite NASA TRMM - LIS
- Intensità delle precipitazioni: campagna internazionale di
misura a Vigna di Valle organizzata dal Ser ...
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No.10 - November 2010
is an issue of iLEAPS Newsletter. iLEAPS, 2011The latest iLEAPS Newsletter No. 10 deals with "Terrestrial feedbacks and Earth system models".
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CAWCR technical report, 43. Exploring the co-benefit of electric vehicle uptake and ozone pollution reduction in Sydney - Final report.
Given the likely pace of change in the electric vehicle market, it is important that the environmental externalities are identified and quantified. In this report we present the results of a modelling study which investigated how ozone pollution in the Greater Metropolitan Region of Sydney NSW, Australia would respond to the replacement of Sydney’s internal combustion engine (ICE) passenger vehicle fleet with a fleet of electric vehicles. A brief description of the modelling methodology is provided in the next section, and a summary of the modelling outcomes is provided in the following sectio ...
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International Polar Year (IPY). Understanding Earth's Polar challenges : International Polar Year 2007-2008 - summary by the IPY Joint Committee
The International Polar Year (IPY) 2007–2008, co-sponsored by ICSU and WMO, became the largest coordinated research program in the Earth’s polar regions, following in the footsteps of its predecessor, the first and second International Polar Years in 1881-1883 and 1932-1933 and the International Geophysical Year 1957–1958.
An estimated 50,000 researchers, local observers, educators, students, and support personnel from more than 60 nations were involved in the 228 international IPY projects (170 in science, 1 in data management, and 57 in education and outreach) and related national eff ...
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CAWCR technical report, 44. Composition of the atmosphere - abstracts of the fifth CAWCR Workshop 15 November - 17 November 2011, Melbourne, Australia
The aims of the meeting are to: 1) understand the role of atmospheric chemistry and composition in global atmospheric change as expressed in the Australasian region and internationally; and 2) to provide a forum for atmospheric composition researchers from different disciplines (in-situ observations, remote sensing observations, modelling) to share ideas, enhance collaboration and develop a coordinated regional approach to characterising atmospheric processes in Australasia.
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GAW Report, 200. WMO/GAW Standard Operating Procedures for In-situ Measurements of Aerosol Mass Concentration, Light Scattering and Light Absorption
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WMO Strategic Plan 2012-2015
The WMO Strategic Plan is the result of an organization-wide strategic, operational and budgeting process to provide a blueprint for the 188 Member States and Territories to meet the changing needs of their communities for weather, climate, water and related environmental information.
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Prediction from Weeks to Decades
This white paper is a synthesis of several recent workshops, reports and published literature: (Smith et al., 2011; Anderson et al. 2011; Weller et al. 2010; Meehl et al. 2009; Hurrell et al. 2009; Shukla et al. 2010 and Brunet et al. 2010). The intent is to document: (i) the scientific basis for prediction from weeks to decades; (ii) current capabilities; and (iii) outstanding challenges. We focus on time--‐scales from beyond the time scale of deterministic weather (i.e., sub--‐seasonal) to decadal.
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Reconciling anthropogenic climate change with observed temperature 1998–2008
Given the widely noted increase in the warming effects of rising greenhouse gas concentrations, it has been unclear why global surface temperatures did not rise between 1998 and 2008. We find that this hiatus in warming coincides with a period of little increase in the sum of anthropogenic and natural forcings. Declining solar insolation as part of a normal eleven-year cycle, and a cyclical change from an El Nino to a La Nina dominate our measure of anthropogenic effects because rapid growth in short-lived sulfur emissions partially offsets rising greenhouse gas concentrations. As such, we fin ...
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Report on the activities of the wintering party of the 49th Japanese Antarctic Research Expedition in 2008-2009
Antarctic Record, Vol. 54, No. 2. Ushio Shuki - Scholarly and Academic Information Navigator (CiNii), 2010The wintering party of the 49th Japanese Antarctic Research Expedition (JARE-49), consisting of 29 members, was conducted as the second year of the 7th four-year plan of JARE and the second half of the International Polar Year 2007-2008 (IPY2007-2008) at Syowa Station and its surrounding areas. JARE-49 took over management of the station facilities and functions from JARE-48 on February 1, 2008, and performed scientific observations and logistic duties. Though it was a little smaller in terms of number of wintering personnel than previous teams, it was well prepared to perform station manageme ...
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Simulation of the Bare Soil Surface Energy Balance at the Tongyu Reference Site in Semiarid Area of North China
The performance of a 1-D soil model in a semiarid area of North China was investigated using observational data from a cropland station at the Tongyu reference site of the Coordinated Enhanced Observing Period (CEOP) during the non-growing period, when the ground surface was covered with bare soil. Comparisons between simulated and observed soil surface energy balance components as well as soil temperatures and water contents were conducted to validate the soil model. Results show that the soil model could produce good simulations of soil surface temperature, net radiation flux and sensible he ...
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Assessing the Impacts of Eurasian Snow Conditions on Climate Predictability with a Global Climate Model
On the basis of two ensemble experiments conducted by a general atmospheric circulation model (Institute of Atmospheric Physics nine-level atmospheric general circulation model coupled with land surface model, hereinafter referred to as IAP9L_CoLM), the impacts of realistic Eurasian snow conditions on summer climate predictability were investigated. The predictive skill of sea level pressures (SLP) and middle and upper tropospheric geopotential heights at mid-high latitudes of Eurasia was enhanced when improved Eurasian snow conditions were introduced into the model. Furthermore, the model ski ...
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